Journal of Primeasia

Integrative Disciplinary Research | Online ISSN 3064-9870 | Print ISSN 3069-4353
570
Citations
221.2k
Views
147
Articles
Your new experience awaits. Try the new design now and help us make it even better
Switch to the new experience
REVIEWS   (Open Access)

From Mine to Material Loop: A Systematic Review and Meta-Analysis of Lithium Recovery Efficiency, Global Warming Potential, and Life Cycle Methodological Variability in Spent Lithium-Ion Battery Recycling

Abstract 1. Introduction 2.  Materials and Methods 3. Results 4.Discussion 5. Limitations 6. Conclusion References

Hussein Naser Radhi 1*

+ Author Affiliations

Journal of Primeasia 7 (1) 1-8 https://doi.org/10.25163/primeasia.7110789

Submitted: 02 May 2026 Revised: 22 June 2026  Accepted: 30 June 2026  Published: 01 July 2026 


Abstract

Lithium-ion batteries sit at the heart of the clean energy transition — and yet, the way we extract, use, and discard them raises uncomfortable questions that the field hasn't fully resolved. This systematic review and meta-analysis attempts to cut through that complexity, drawing on peer-reviewed studies to compare the environmental performance of lithium recovery from spent batteries against conventional primary mining. We focused specifically on global warming potential (GWP), process-level recovery efficiency, and the often-overlooked role of life cycle impact assessment (LCIA) methodology in shaping what the data actually tell us. What emerged was, frankly, a messier picture than the headlines suggest. Recovery rates ranged from 91.6% to 99.0% — a pooled mean of 96.4% ± 0.9% — but that spread matters. Closed-loop hydrometallurgical routes performed most consistently; selective acid leaching, less so. GWP estimates varied even more dramatically, from 2.31 to 12.50 kg CO2e per kg of cathode active material, depending almost entirely on where the electricity came from. That finding alone deserves more attention than it typically receives. Across methodologies, recycled lithium reliably outperformed primary production on climate metrics — but only when paired with low-carbon energy. Functional unit choice and system boundary definitions shifted conclusions more than most studies acknowledge. These aren't merely technical footnotes; they're the variables that determine whether recycling actually delivers on its environmental promise.

Keywords: Lithium recycling; Life cycle assessment; Global warming potential; Cathode active materials; Meta-analysis; Battery sustainability

References

Ajiboye, A. E., & Dzwiniel, T. L. (2023). Sequential recovery of critical metals from leached liquor of spent lithium-ion batteries. Batteries, 9(11), 549. https://doi.org/10.3390/batteries9110549

Ali, S. H., Giurco, D., Arndt, N., et al. (2017). Mineral supply for sustainable development requires resource governance. Nature, 543(7645), 367–372. https://doi.org/10.1038/nature21359

Barman, P., et al. (2023). Electric vehicle battery supply chain and critical materials. Energies, 16(8), 3369. https://doi.org/10.3390/en16083369

Blömeke, S., Scheller, C., Cerdas, F., Thies, C., Hachenberger, R., Gonter, M., & Spengler, T. S. (2022). Material and energy flow analysis for environmental and economic impact assessment of industrial recycling routes for lithium-ion traction batteries. Journal of Cleaner Production, 377, 134344. https://doi.org/10.1016/j.jclepro.2022.134344

Bobba, S., et al. (2019). How will second-use of batteries affect stocks and flows in the EU? Resources, Conservation and Recycling, 145, 262–273. https://doi.org/10.1016/j.resconrec.2019.02.022

Borenstein, M., Hedges, L. V., Higgins, J. P. T., & Rothstein, H. R. (2009). Introduction to meta-analysis. Wiley. https://doi.org/10.1002/9780470743386

Cerdas, F., et al. (2018). Exploring the effect of increased energy density on environmental impacts. Energies, 11(1), 150. https://doi.org/10.3390/en11010150

Chan, K. H., Anawati, J., Malik, M., & Azimi, G. (2021). Closed-loop recycling of lithium, cobalt, nickel, and manganese from waste lithium-ion batteries of electric vehicles. ACS Sustainable Chemistry & Engineering, 9(12), 4398–4410. https://doi.org/10.1021/acssuschemeng.0c06869

Chen, W.-S., & Ho, H.-J. (2018). Recovery of valuable metals from NMC cathode waste. Metals, 8(5), 321. https://doi.org/10.3390/met8050321

Ciez, R. E., & Whitacre, J. F. (2019). Examining different recycling processes for lithium-ion batteries. Nature Sustainability, 2(2), 148–156. https://doi.org/10.1038/s41893-019-0222-5

Dar, A. A., et al. (2025). Sustainable extraction of critical minerals from waste batteries. Batteries, 11(2), 51. https://doi.org/10.3390/batteries11020051

DerSimonian, R., & Laird, N. (1986). Meta-analysis in clinical trials. Controlled Clinical Trials, 7(3), 177–188. https://doi.org/10.1016/0197-2456(86)90046-2

Doose, S., et al. (2021). Challenges in eco-friendly battery recycling. Metals, 11(2), 291. https://doi.org/10.3390/met11020291

Egger, M., Davey Smith, G., Schneider, M., & Minder, C. (1997). Bias in meta-analysis detected by a simple, graphical test. BMJ, 315(7109), 629–634. https://doi.org/10.1136/bmj.315.7109.629

European Commission. (2017). Study on the review of the list of critical raw materials. https://ec.europa.eu/docsroom/documents/25181

European Commission. (2023). Study on the critical raw materials for the EU 2023–Final report. https://single-market-economy.ec.europa.eu/sectors/raw-materials/areas-specific-interest/critical-raw-materials_en https://doi.org/10.56181/ETUQ3384

Ferro, P., & Bonollo, F. (2019). Design for recycling in a critical raw materials perspective. Recycling, 4(4), 44. https://doi.org/10.3390/recycling4040044

Geissdoerfer, M., et al. (2017). The circular economy—A new sustainability paradigm? Journal of Cleaner Production, 143, 757–768. https://doi.org/10.1016/j.jclepro.2016.12.048

Gielen, D. (2021). Critical minerals for the energy transition. IRENA. https://irena.org

Global Battery Alliance. (2020). A vision for a sustainable battery value chain in 2030. https://www.weforum.org

Gonzales-Calienes, G., et al. (2023). Economic and environmental viability of lithium-ion battery recycling. Batteries, 9(7), 375. https://doi.org/10.3390/batteries9070375

Harper, G., et al. (2019). Recycling lithium-ion batteries from electric vehicles. Nature, 575(7781), 75–86. https://doi.org/10.1038/s41586-019-1682-5

Helms, H., et al. (2016). Weiterentwicklung und vertiefte Analyse der Umweltbilanz von Elektrofahrzeugen. Umweltbundesamt. https://www.umweltbundesamt.de

Higgins, J. P. T., Thomas, J., Chandler, J., Cumpston, M., Li, T., Page, M. J., & Welch, V. A. (2022). Cochrane handbook for systematic reviews of interventions (Version 6.3). Cochrane. http://www.training.cochrane.org/handbook

Higgins, J. P. T., Thompson, S. G., Deeks, J. J., & Altman, D. G. (2003). Measuring inconsistency in meta-analyses. BMJ, 327(7414), 557–560. https://doi.org/10.1136/bmj.327.7414.557

Hofmann, M., et al. (2018). Critical raw materials: A perspective from materials science. Sustainable Materials and Technologies, 17, e00074. https://doi.org/10.1016/j.susmat.2018.e00074

International Energy Agency. (2023). World energy outlook 2023. https://www.iea.org/reports/world-energy-outlook-2023

Islam, M. T., & Iyer-Raniga, U. (2022). Lithium-ion battery recycling in the circular economy. Recycling, 7(3), 33. https://doi.org/10.3390/recycling7030033

Kallitsis, E., Korre, A., & Kelsall, G. H. (2022). Life cycle assessment of recycling options for automotive Li-ion battery packs. Journal of Cleaner Production, 371, 133636. https://doi.org/10.1016/j.jclepro.2022.133636

Kawajiri, K., Tahara, K., & Uemiya, S. (2022). Lifecycle assessment of critical material substitution. Resources, Environment and Sustainability, 7, 100047. https://doi.org/10.1016/j.resenv.2022.100047

Løvik, A. N., Hagelüken, C., & Wäger, P. (2018). Improving supply security of critical metals. Sustainable Materials and Technologies, 15, 9–18. https://doi.org/10.1016/j.susmat.2018.01.003

Lu, Z., Ning, L., Zhu, X., & Yu, H. (2025). Critical pathways for transforming the energy future: A review of innovations and challenges in spent lithium battery recycling technologies. Materials, 18(13), 2987. https://doi.org/10.3390/ma18132987

Mahnoor, M., et al. (2025). Critical and strategic raw materials for energy storage devices. Batteries, 11(4), 163. https://doi.org/10.3390/batteries11040163

Martin, N., et al. (2022). New techniques for assessing critical raw material aspects. Environmental Science & Technology, 56, 17236–17245. https://doi.org/10.1021/acs.est.2c05308

Martinez-Laserna, E., et al. (2018). Battery second life: Hype, hope or reality? Renewable and Sustainable Energy Reviews, 93, 701–718. https://doi.org/10.1016/j.rser.2018.04.035

McKerracher, C. (2019). Electric vehicle outlook 2019. BloombergNEF. https://about.bnef.com

Mohr, M., Peters, J. F., Baumann, M., & Weil, M. (2020). Toward a cell-chemistry specific life cycle assessment of lithium-ion battery recycling processes. Journal of Industrial Ecology, 24(6), 1310–1322. https://doi.org/10.1111/jiec.13021

Neidhardt, M., et al. (2022). Forecasting the global battery material flow. Applied Sciences, 12(9), 4790. https://doi.org/10.3390/app12094790

Olsson, L., et al. (2018). Circular business models for extended EV battery life. Batteries, 4(4), 57. https://doi.org/10.3390/batteries4040057

Page, M. J., McKenzie, J. E., Bossuyt, P. M., Boutron, I., Hoffmann, T. C., Mulrow, C. D., et al. (2021). The PRISMA 2020 statement: An updated guideline for reporting systematic reviews. BMJ, 372, n71. https://doi.org/10.1136/bmj.n71

Peng, C., Liu, F., Wang, Z., Wilson, B. P., & Lundström, M. (2019). Selective extraction of lithium (Li) and preparation of battery grade lithium carbonate (Li2CO3) from spent Li-ion batteries in nitrate system. Journal of Power Sources, 415, 179–188. https://doi.org/10.1016/j.jpowsour.2019.01.072

Peters, J. F., & Weil, M. (2016). A critical assessment of the resource depletion potential of LIBs. Resources, 5(4), 46. https://doi.org/10.3390/resources5040046

Pommeret, A., Ricci, F., & Schubert, K. (2022). Critical raw materials for the energy transition. European Economic Review, 141, 103991. https://doi.org/10.1016/j.euroecorev.2021.103991

Rapier, R. (2024). Breaking records: 2024 statistical review of world energy highlights. Forbes. https://www.forbes.com

Sato, F. E. K. S., & Nakata, T. (2020). Recoverability analysis of critical materials from EV LIBs in Japan. Sustainability, 12(1), 147. https://doi.org/10.3390/su12010147

Skrzekut, T., Piotrowicz, A., Noga, P., Wedrychowicz, M., & Bydalek, A. W. (2022). Studies of selective recovery of zinc and manganese from alkaline batteries scrap by leaching and precipitation. Materials, 15(11), 3966. https://doi.org/10.3390/ma15113966

Tawonezvi, T., et al. (2023). Recovery and recycling of valuable metals from spent LIBs. Energies, 16(3), 1365. https://doi.org/10.3390/en16031365

Velázquez-Martínez, O., et al. (2019). A critical review of lithium-ion battery recycling processes. Batteries, 5(4), 68. https://doi.org/10.3390/batteries5040068

Wang, W.-Y., et al. (2020). Recovery of cobalt and nickel from NMC LIBs. Minerals, 10(7), 662. https://doi.org/10.3390/min10080662

Zhang, G., Yuan, X., He, Y., Wang, H., Zhang, T., & Xie, W. (2021). Recent advances in pretreating technology for recycling valuable metals from spent lithium-ion batteries. Journal of Hazardous Materials, 406, 124332. https://doi.org/10.1016/j.jhazmat.2020.124332


Article metrics
View details
0
Downloads
0
Citations
1
Views

View Dimensions


View Plumx


View Altmetric



0
Save
0
Citation
1
View
0
Share